Evolution of alpha-pinene oxidation products in the presence of varying oxidizers: CI- APi-TOF point of view

نویسندگان

  • Matti P. Rissanen
  • Tuija Jokinen
  • Siegfried Schobesberger
  • Arnaud P. Praplan
  • Mikko Sipilä
  • Nina Sarnela
  • Heikki Junninen
  • Jonathan Duplissy
  • Juha Kangasluoma
  • Jani Hakala
  • Daniela Wimmer
  • Alexey Adamov
  • Katrianne Lehtipalo
  • Tuomo Nieminen
  • Markku Kulmala
  • Douglas R. Worsnop
چکیده

Alpha-pinene oxidation was studied in the CERN CLOUD chamber under near atmospheric conditions using varying levels of different oxidizers (i.e., O3, HOx and NOx with differing gas mixture compositions) in the presence and absence of UV-radiation, SO2 and additional organic traces; ammonia (NH3) and dimethylamine (DMA). The oxidation products and their evolution due to aging in the chamber were studied using a novel CI-APi-TOF technique, with the nitrate ion (NO3 ) based chemical ionization (CI) scheme. We aimed to the results that would indicate how different oxidizing pathways lead to different product distributions in the product clusters detected.

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تاریخ انتشار 2016